Chem. Sci., 2025, Accepted Manuscript DOI: 10.1039/D5SC06866E, Edge Article J. Benji Rowlands, Lina Jonsson, Jonathan Goodman, Peter Howe, Werngard Czechtizky, Tomas Leek, Richard James Lewis Human interpretation of spectroscopic data remains key to confirming newly synthesised chemical structures. Whilst there have been advances in automated spectral interpretation, the false positive and false negative rates remain...